The Shins and Wilco are two incredible bands. Wilco's Yankee Hotel Foxtrot is an absolute masterpiece. That said, I think "They'll Soon Discover" edges it out!
The original movie soundtrack was soo good! I'm disappointed that Sponge Out of Water didn't have a great soundtrack (or really much of a soundtrack at all). Hoping that the third movie gets artists as great as the first movie.
Psychic Wall for sure, runners up would be You Better Swim (I mean, Motorhead on SpongeBob, and it actually works! :P) Under My Rock, and They'll Soon Discover.
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